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You can simulate a Screenshot on our Virtual Machines for both Android and iPhone
For Android
Visit the Console screen
Hit Enter > Run
input keyevent KEYCODE_SYSRQ
This will simulate a Screenshot. The image will be stored in Photos

For iPhone
You have the ability to take screenshots utilizing the AssistiveTouch option from the interface of the virtual machine. Please take a look at this helpful Corellium Support article regarding Holding Down Two Virtual Hardware Buttons.